Optimal mapping of terrestrial gamma dose rates using geological parent material and aerogeophysical survey data

Regulatory authorities need ways to estimate natural terrestrial gamma radiation dose rates (nGy h−1) across the landscape accurately, to assess its potential deleterious health effects. The primary method for estimating outdoor dose rate is to use an in situ detector supported 1 m above the ground, but such measurements are costly and cannot capture the landscape-scale variation in dose rates which are associated with changes in soil and parent material mineralogy. We investigate the potential for improving estimates of terrestrial gamma dose rates across Northern Ireland (13542 km2) using measurements from 168 sites and two sources of ancillary data: (i) a map based on a simplified classification of soil parent material, and (ii) dose estimates from a national-scale, airborne radiometric survey. We used the linear mixed modelling framework in which the two ancillary variables were included in separate models as fixed effects, plus a correlation structure which captures the spatially correlated variance component. We used a cross-validation procedure to determine the magnitude of the prediction errors for the different models. We removed a random subset of 10 terrestrial measurements and formed the model from the remainder (n = 158), and then used the model to predict values at the other 10 sites. We repeated this procedure 50 times. The measurements of terrestrial dose vary between 1 and 103 (nGy h−1). The median absolute model prediction errors (nGy h−1) for the three models declined in the following order: no ancillary data (10.8) > simple geological classification (8.3) > airborne radiometric dose (5.4) as a single fixed effect. Estimates of airborne radiometric gamma dose rate can significantly improve the spatial prediction of terrestrial dose rate

Radiometric Flight Trials in the Forth Estuary on 7/8/91

A brief radiometric flight trial was undertaken on 7th August 1991, essentially to prove a new gamma spectrometry installation. A twin engined helicopter operated by Dollar helicopters out of Cumbernauld Airport was used for the exercise. The new equipment under test comprised (i) a spectrometer mounting plate manufactured by Dollar to take SURRC equipment for rapid deployment, (ii) a 19" rack mounted spectrometer incorporating proven SURRC components, but with additional duplex inverter based UPS, and (iii) a Navstar XR4 GPS system with aircraft patch type aerial. The flight trial was conducted in the Forth Estuary area focussing on three small sites of incidental interest

An Aerial Gamma Ray Survey of Springfields and the Ribble Estuary in September 1992

<p>A short aerial gamma ray survey was conducted in the vicinity of the Springfields site and Ribble Estuary from 1st-5th September 1992, to define existing background radiation levels, against which any future changes can be assessed. A twin engine AS 355 "Squirrel" helicopter chartered from Dollar Helicopters was used for this work. It was loaded with a 16 litre NaI(Tl) gamma ray detector and spectroscopy system on the 31st August and during the following days over 2700 separate spectra were recorded within a survey area of 20 x 12 km. Gamma ray spectra were recorded every 5 seconds at survey speed and altitude of 120 kph and 75 m respectively. A flight line spacing of 0.3km was chosen for the main survey area. On the 3rd September a low altitude, high spatial resolution (flight line spacing 100m and altitude 30m) was made over Banks Marsh (an area frequented by local wild fowlers).</p> <p>Survey results have been stored archivally and used to map the naturally occurring radionuclides 40K, 214Bi and 208Tl together with 137Cs and total gamma ray flux. In addition, for the first time, estimates of 234mPa in terms of deconvoluted count rate (normalised to 100m altitude) were made in the presence of 228Ac interference probably in disequilibrium with its parent thorium series.</p> <p>The maps provide a clear indication of the distribution and sources of environmental radioactivity in the Ribble at the time of the survey. The Ribble estuary is subject to regular and ongoing ground based studies by BNF, MAFF, HMIP, and University based groups, as a result of the authorised discharges of low level radioactivity from the Springfields site. The results of this survey complement this ground based work, and add to confidence that the estuarine system, it's associated sediments, tide washed pastures, salt marshes and river banks, have been thoroughly examined. There is support for earlier conclusions that the Cs on the salt marshes is the dominant source of external gamma exposure, and that the Springfields contribution to these locations is minor in comparison with this, Sellafield derived, signal. Upstream the situation is more complex, particularly where the dynamic sources of beta radiation are considered. As far as critical group assessments are concerned the survey provides clear evidence that the areas affected by 137Cs, where external gamma dose and possible food chain effects are of greatest interest, are in the lower reaches of the Ribble, whereas, at the time of the survey the 234mPa distribution was in the upper reaches of the river. This not only confirms the findings of ground based work, but provides some assurance that the different exposure paths (external gamma dose, skin dose) are not entirely synergistic. The discovery of possible transient sources of natural 228Ac in the salt marsh environment as a consequence of Th series disequilibrium immediately following spring tides is extremely interesting. If substantiated by further studies using semiconductor detectors this provides a new insight into the dynamic radiation environment of tide washed contexts.</p> <p>Aerial survey can potentially provide a rapid and cost effective means of studying environmentally dynamic sources such as 234mPa. In the case of the Ribble it would be necessary to reduce survey height to below 50m ground clearance to improve spatial resolution. Possible inconvenience to residents and property owners of such low altitude flights would have to be considered in addition to the potential value of environmental knowledge of the behaviour of short lived nuclides in a dynamic system such the Ribble estuary. There is nonetheless considerable potential for time series studies of this location. Recent flight trials by SURRC incorporating high efficiency germanium semiconductor detectors have verified the feasibility and potential a hybrid scintillation⁄ semiconductor spectrometer. Such a device can resolve any ambiguities arising from overlapping gamma ray peaks. This is particularly relevant to the confirmation of 228Ac in salt marshes. Ground based sampling at the time of measurement would enable concentration calibrations to be made for these dynamic sources. Further ground based measurements would be desirable to establish the extent to which low energy photons contribute to external gamma ray dose rates from sources with pronounced subsurface activity maxima.</p&gt

An Airborne Gamma Ray Survey of Parts of SW Scotland in February 1993. Final Report

An airborne gamma ray survey was conducted for the Scottish Office Environment Department of coastal and inland parts of SW Scotland to define existing background levels, to locate features worthy of further attention, and to demonstrate the emergency response capabilities of radiometric methods. Coastal areas were surveyed with 500 m line spacing. Inland areas were specified to 2 km line spacing, however it was possible to achieve 1 km line spacing in the majority of the inland zone. Fieldwork was conducted between the 1st and 16th February 1993. A total of over 17,000 gamma ray spectra were recorded, using a 16 litre NaI spectrometer mounted in a helicopter flying at 50-75m ground clearance and 120kph. A total area of 3650 km2 was surveyed in 41.6 flying hours, from roughly 4370 line kilometres. The data were reduced in the field using standard SURRC procedures for background subtraction, stripping of spectral interferences, altitude correction, and calibration. Preliminary maps of the distribution of 137Cs, 40K, 214Bi, 208Tl, and estimated ground level gamma dose rate were produced during the fieldwork period using working calibration values derived from previous surveys. A set of core samples was collected from Wigtown Merse, Longbridgemuir and Caerlaverock merse for calibration purposes, and aerial observations were performed at these sites. Further soil sampling and ground level in-situ gamma spectrometry was performed in the summer of 1993 to investigate the applicability of the calibration to a range of upland soil types and topographical environments. These locations received peak deposition from the Chernobyl accident, are vulnerable to wet deposition, and are difficult to monitor rapidly using ground based methods. A total of 76 soil cores, subdivided into 168 separate samples was thus collected for high resolution gamma spectrometry in the laboratory. This was conducted from April to November 1993. For the terrestrial sites the aerial survey estimates based on the working calibration, were in good agreement with both in-situ gamma spectrometry and the results of core analysis. This validates the preliminary maps in these contexts, and confirms that a general calibration is sufficient for fallout mapping under emergency response conditions. On coastal salt marsh sites (merse), where aged deposits of Sellafield derived activity have accumulated, subsurface activity profiles for 137Cs and 241Am and the presence of superficial levels of 134Cs were observed from the soil cores. Similar features have been observed in previous surveys. In these cases the effects of source burial must be taken into account to avoid underestimation of activity levels by both ground-based and aerial gamma spectrometry. A separate set of detailed maps for the principal merse sites was therefore prepared using a calibration factor derived from the soil cores from this context. There are prospects for developing spectral analysis procedures to account for source depth in aerial surveys. Source burial on the merse also has implications for sampling techniques, and for dose rate measurement, which would merit further consideration. The radiometric maps show clearly the distributions of each individual nuclide and indicate the contribution which individual localised features make to the overall gamma ray dose rate. Naturally occurring nuclides reflect the underlying geological and geomorphological contexts of the landscape. The main granite intrusions, most notably at Cairnsmore of Fleet, the Loch Doon Granodiorite, Glencairn of Carsphairn, the Dalbeattie granite, and Criffel Pluton are readily visible in 40K, 214Bi and 208Tl maps, and control their local radiation environments. A number of areas of enhanced 214Bi, which may reflect radon potential, were noted. A transient radon associated 214Bi signal was observed on the west of the Wigtown peninsular during the survey. Examination of spectral data in the vicinity of Dundrennan has confirmed that there is no evidence of widespread terrestrial contamination arising from the use of depleted uranium projectiles on the range. The 137Cs map indicates the environmental distribution of this nuclide in considerable detail. Levels of 137Cs range from approximately 2 kBq m-2, a level consistent with global weapons’ testing fallout, from 2-40kBq m-2 on terrestrial sites affected by deposition from the Chernobyl accident, and from 40 kBq m-2 to over 200 kBq m-2 on tide washed pastures which have accumulated marine sediments from the Irish Sea. All three levels are represented within the survey zone, in a manner which is consistent with the findings of previous aerial surveys in adjacent areas, and with ground based studies. The main Chernobyl deposition in Dumfries and Galloway appears to have occurred between an area just east of the Nith, and Glenluce. The northern limit has not yet been defined, and there may be grounds for considering extension of the northern and particularly eastern limits of the inland survey zone. Within the survey zone the deposition pattern is complex, including both upland and lowland components. The plume trajectories for deposition inferred from these observations are oriented northwards rather than in the NW directions predicted by meteorological derived estimates. This may explain the contradiction between results from the Central Highlands and the estimated fallout patterns. The data presented here both add to previous knowledge, and serve as a baseline against which any future changes can be measured. The survey provides systematic coverage of the sedimentary and terrestrial coastal system for the first time, and has identified a number of merse sites which have accumulated radioactivity from past marine discharges from Sellafield, and which are not routinely monitored under existing Scottish Office arrangements. Some of these locations are extensive and fall within SSI’s; furthermore they are key sites for studying future deposition trends. It would seem prudent to review radiological assessments in the light of this work to ensure that the patterns of occupancy and sensitive ecologies of the merse are taken fully into account. The emergency response potential of aerial radiometrics has been clearly demonstrated in this project. It provides the only practical means of providing comprehensive environmental measurements of remote and upland landscapes on a short time scale, with an effective area sampling density some 106-107 times greater than soil sampling. Results are compatible with ground based approaches, and could focus ground based efforts effectively under emergency conditions. Modern approaches to data recording and analysis are able to produce maps during the survey period. National baseline mapping in Scotland, at 1 km resolution, would require less than 800 flying hours; 20 km line spacing would take roughly 40 hours of flight time. A long term programme of high resolution national baseline mapping, coupled to an emergency response standby arrangement, would provide an extremely cost effective way of preserving the capability developed since the Chernobyl accident, while producing high quality environmental data for research purpos

An Airborne Gamma Ray Survey of Three Ayrshire Districts

<p>An aerial radiometric survey of Cunninghame, Kilmarnock and Loudon and Kyle and Carrick districts was conducted by SURRC from July 16th to 2nd August 1990. A 16 litre NaI spectrometer was used to map the distribution of radiation from 137Cs, 40K, 214Bi, 208Tl, and also to estimate the total gamma dose rate from all sources over an area of 2500 km2. A helicopter, chartered from PLM (Inverness), was used to survey the districts at a height of 100m above ground, flight lines being spaced by approximately 1 km and oriented north-south within the study zone.</p> <p>More than 6000 gamma ray spectra were recorded in the survey. Integrated count rates for each nuclide have been collated and calibrated to ground level area inventories based on a comparison between airborne and terrestrial gamma fluxes over sites of known radioactivity. Extensive field based studies were conducted in parallel with the aerial survey to support the calibration. Detailed colour contour maps show the distribution of radionuclides with roughly 1 km resolution throughout the area.</p> <p>The survey is intended to provide a comprehensive baseline against which any future changes can be measured. In the event of any future nuclear accident it will be possible to state clearly what has been added to the existing background.</p> <p>The variations in natural background sources have been defined and can be related to underlying geological features. Granite masses in the north of Arran and SW of Loch Doon show elevated levels of potassium, 214Bi (denoting post-radon uranium series activity) and 208Tl (from the decay of thorium). By contrast the ultrabasic rocks which occur on the mainland in all three districts show natural radioactivity levels between 5 and 10 times lower. Sandstone areas give intermediate results. 214Bi is a radon daughter product which may be of value in indicating the variation in radon source term underlying domestic problems.</p> <p>137Cs has been mapped in detail. Peak fallout occurs principally in the SE of Kyle and Carrick (> 25 kBq m-2), in parts of central Arran (> 15 kBq m-2), and more generally inland (> 10 kBq m-2). Some coastal areas have been virtually unaffected by Chernobyl. Marine 137Cs was detected notably on salt marshes near to the Irvine racecourse and on the Western coast of Great Cumbrae. Part of this inventory derives probably from Sellafield, and perhaps from Hunterston. Local sampling programmes here would be of interest. Close to the Hunterston “A” power station a small area with over 10 times natural gamma activity was encountered by helicopter. Scottish Nuclear were informed of these findings and conducted a prompt ground level investigation to identify the source of the activity, associated with an obsolete precipitator plant. This source of activity will be removed during decommissioning, and it is suggested that a repeat survey be conducted once this has been done.</p> <p>Despite the presence of readily measurable anthropogenic sources in many parts of the three districts the overall environmental quality appears to be high. Natural sources account for the majority of the measured gamma ray dose rates, and the higher activity rock types apparently occur in sparsely populated zones. Follow up studies to examine further details of these patterns at ground level, and to itigate domestic and urban contexts wouldvaluable. The archival results generated in this projreprese useful resource for such studies, and asecure the possibility of detecting future changes he event of anident involving significant quantities odioactivity.</p&gt

Testing Logselfsimilarity of Soil Particle Size Distribution: Simulation with Minimum Inputs

Particle size distribution (PSD) greatly influences other soil physical properties. A detailed textural analysis is time-consuming and expensive. Soil texture is commonly reported in terms of mass percentages of a small number of size fractions (typically, clay, silt and sand). A method to simulate the PSD from such a poor description or even from the poorest description, consisting in the mass percentages of only two soil size fractions, would be extremly useful for prediction purposes. The goal of this paper is to simulate soil PSDs from the minimum number of inputs, i.e., two and three textural fraction contents, by using a logselfsimilar model and an iterated function system constructed with these data. High quality data on 171 soils are used. Additionally, the characterization of soil texture by entropy-based parameters provided by the model is tested. Results indicate that the logselfsimilar model may be a useful tool to simulate PSD for the construction of pedotransfer functions related to other soil properties when textural information is limited to moderate textural data